Ionic Liquids As Green Solvents Progress and Prospects

, by Rogers, Robin D.; Seddon, Kenneth R.

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ISBN: 9780841238565 | 0841238561
Cover: Hardcover
Copyright: 9/25/2003

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Following Ionic Liquids: Industrial Applications to Green Chemistry, SS #818 , by the same editors, this book focuses on exciting new developments in ionic liquids.

Preface

xiii

Overview

1. Selection of Ionic Liquids for Green Chemical Applications

(12)

John D. Holbrey, Megan B. Turner, and Robin D. Rogers

Ionic Liquids: Manufacture and Synthesis

2. Ionic Liquids: Improved Syntheses and New Products

(18)

Adrian J. Carmichael, Maggel Deetlefs, Martyr J. Earle, Ute Fröhlich, and Kenneth R. Seddon

3. Challenges to the Commercial Production of Ionic Liquids

(9)

Philip E. Rakita

4. Industrial Preparation of Phosphonium Ionic Liquids

(16)

Christine J. Bradaric, Andrew Dovenard, Christine Kennedy, Allan J. Robertson, and Yuehui Zhou

5. New Ionic Liquids Based on Alkylsulfate and Alkyl Oligoether Sulfate Anions: Synthesis and Applications

(13)

Peter Wasserscheid, Roy van Hal, Andreas Bösmann, Jochen Eßer, and Andreas Jess

6. Green Synthesis of Ionic Liquids for Green Chemistry

(12)

Rex X. Ren

7. Expeditious Synthesis of Ionic Liquids Using Ultrasound and Microwave Irradiation

(11)

Kajender S. Varma.

8. Unprecedented Synthesis of 1,3-dialkylimidazolium-2-carboxylate: Applications in the Synthesis of Halogen-Free Ionic Liquids and Reactivity as Carbon Dioxide Transfer Agent to Active C-H Bonds

(7)

M. Aresta, I. Tkatchenko, and I. Tommasi

9. Commercially Available Salts as Building Blocks for New Ionic Liquids

100

(10)

James H. Davis, Jr, and Phillip A. Fox

Characterization and Engineering

10. Phase Equilibria of Gases and Liquids with 1-n-butyl-3-Methylimidazolium Tetrafluoroborate

110

(11)

Jennifer L. Anthony, Jacob M. Crosthwaite, Daniel G. Hert, Sudhir N. V. K. Aki, Edward J. Magien, and Joan F. Brennecke

11. Heat Capacities of Ionic Liquids and Their Applications as Thermal Fluids

121

(13)

John D. Holbrey, W. Matthew Reichert, Ramana G. Reddy, and Robin D. Rogers

12. Thermodynamic Properties of Liquid Mixtures Containing Ionic Liquids

134

(17)

Andreas Heintz, Jochen K. Lehmann, and Sergey P. Verevkin

13. Liquid and Solid-State Structures of 1,3-Dimethylimidazolium Salts

151

(11)

D. T. Bowron, C. Hardacre, J. D. Holbrey, S. E, J. McMath, M. Nieuwenhuyzen, and A. K. Soper

14. Molecular Structure of Various Ionic Liquids from Gas Phase Ab Initio Calculations

162

(12)

Timothy I. Morrow and Edward J. Maginn

15. Transition Structure Models of Organic Reactions in Chloroaluminate Ionic Liquids: Cyclopentadiene and Methyl Acrylate Diels-Alder Reaction in Acidic and Basic Melts of 1-Ethyl-3-methylimidazolium Chloride with Aluminum(III) Chloride

174

(18)

Orlando Acevedo and Jeffrey D. Evanseck

Biotechnology in Ionic Liquids

16. Biotransformations in Ionic Liquids: An Overview

192

(14)

Roger A. Sheldon, F. van Rantwijk, and R. Madeira Lau

17. Enzymatic Condensation Reactions in Ionic Liquids

206

(6)

Nicole Kaftzik, Sebastian Neumann, Maria-Regina Kula, and Udo Kragl

18. Aspects of Chemical Recognition and Biosolvation within Room Temperature Ionic Liquids

212

(13)

Gary A. Baker, Sheila N. Baker, T. Mark McCleskey, and James H. Werner

19. Ionic Liquids Create New Opportunities for Nonaqueous Biocatalysts with Polar Substrates: Acylation of Glucose and Ascorbic Acid

225

(14)

Seongsoon Park, Fredrik Viklund, Karl Hult, and Romas J. Kazlauskas

20. Enzymatic Catalysis in Ionic Liquids and Supercritical Carbon Dioxide

239

(12)

Pedro Lozano, Teresa De Diego, Daniel Carré, Michel Vaultier, and José L. Iborra

21. Efficient Lipase-Catalyzed Enantioselective Acylation in an Ionic Liquid Solvent System

251

(13)

Toshiyuki Itoh, Yoshihito Nishimura, Masaya Kashiwagi, and Makoto Onaka

Non-Catalytic and Calalytic Chemistry

22. Acids and Bases in Ionic Liquids

264

(13)

Douglas R. MacFarlane and Stewart A. Forsyth

23. Catalytic Olefin Epoxidation and Dihydroxylation with Hydrogen Peroxide in Common Ionic Liquids: Comparative Kinetics and Mechanistic Study

277

(12)

Mahdi M. Abu-Omar, Gregory S. Owens, and Armando Durazo

24. Polarity Variation of Room Temperature Ionic Liquids and Its Influence on a Diels-Alder Reaction

289

(11)

Richard A. Bartsch and Sergei V. Dzyuba

25. Polar, Non-Coordinating Ionic Liquids as Solvents for Coordination Polymerization of Olefins

300

(14)

Kevin H. Shaughnessy, Marc A. Klingshirn, Steven J. P'Pool, John D. Holbrey, and Robin D. Rogers

26. The Importance of Hydrogen Bonding to Catalysis in Ionic Liquids: Inhibition of Allylic Substitution and Isomerization by [bmim] [BF4]

314

(9)

James Ross and Jianliang Xiao

27. Recent Developments in the Use of N-Heterocyclic Carbenes: Applications in Catalysis

323

(21)

Rebecca M. Kissling, Mihai S. Viciu, Gabriela A. Grasa, Romain F. Germaneau, Tatyana Güveli, Marie-Christiane Pasareanu, Oscar Navarro-Fernandez, and Steven P. Nolan

Photochemistry

28. An Overview of Photochemistry in Ionic Liquids

344

(7)

Richard M. Pagni

29. Diffusion-Controlled Reactions in Room Temperature Ionic Liquids

351

Charles M. Gordon, Andrew J. McLean, Mark J. Muldoon, and Ian R. Dunkiv

30. Amine Mediated Photoreduction of Aryl Ketones in N-Heterocyclic Ionic Liquids: Novel Solvent Effects Leading to Altered Product Distribution

310

(71)

Paul B. Jones, John L. Reynolds, Robert G. Brinson, and Ryan L. Butke

31. Radiation Chemistry of Ionic Liquids: Reactivity of Primary Species

381

(10)

James F. Wishart

32. Pulse Radiolysis Studies of Reaction Kinetics in Ionic Liquids

391

(19)

P. Neta, D. Behar, and J. Grodkowski

33. Organic Electrochemistry in Ionic Liquids

410

(11)

Andrew P. Doherty and Claudine A. Brooks

34. Solvent Solute Interactions in Ionic Liquid Media: Electrochemical Studies of the Ferricenium-Ferrocene Couple

421

(18)

M. Cristina Lagunas, William R. Pitney, Jan-Albert van den Berg, and Kenneth R. Seddon

35. Electrochemical Studies of Ambient Temperature Ionic Liquids Based on Choline Chloride

439

(14)

Andrew P. Abbott, Glen Capper, David L. Davies, Helen Munro, Raymond K. Rasheed, and Vasuki Tambyrajah

36. Electrodeposition of Nanoscale Metals and Semiconductors from Ionic Liquids

453

(15)

Sherif Zein El Abedin and Frank Endres

Novel Applications

37. Plasticizing Effects of Imidazolium Salts in PMMA: High-Temperature Stable Flexible Engineering Materials

468

(10)

Mark P. Scott, Michael G. Benton, Mustafizur Rahman, and Christopher S. Brazel

38. The Use of Ionic Liquids in Polymer Gel Electrolytes

478

(17)

Hugh C. De Long, Paul C. Trulove, and Thomas E. Sutto

39. Electrochemistry: Ionic Liquid Electroprocessing of Reactive Metals

495

(14)

Jianming Lu and David Dreisinger

40. Electrochemistry: Electrochemically Generated Superoxide Ion in Ionic Liquids: Applications to Green Chemistry

509

(17)

I. M. AlNashef, M. A. Matthews, and J. W. Weidner

41. Conventional Aspects of Unconventional Solvents: Room Temperature Ionic Liquids as Ion-Exchangers and Ionic Surfactants

526

(18)

Mark L. Dietz, Julie A. Dzielawa, Mark P. Jensen, and Millicent A. Firestone

42. Extraction of Chlorophenols from Water Using Room Temperature Ionic Liquids

544

(19)

Evangelia Bekou, Dionysios D. Dionysiou, Ru-Ying Qian, and Gregory D. Botsaris

Indices

Author Index

563

(2)

Subject Index

565

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Ionic Liquids As Green Solvents Progress and Prospects

Summary

Table of Contents

Supplemental Materials